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Werner Uhl, Prof. Dr. - Publications

Affiliations: 
2004-2021 Inorganic Chemistry Westfälische Wilhelms-Universität Münster, Münster, Nordrhein-Westfalen, Germany 
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Year Citation  Score
2021 Brand A, Schulz S, Hepp A, Weigand JJ, Uhl W. Sterically constrained tricyclic phosphine: redox behaviour, reductive and oxidative cleavage of P-C bonds, generation of a dilithium phosphaindole as a promising synthon in phosphine chemistry. Chemical Science. 12: 3460-3474. PMID 34163619 DOI: 10.1039/d0sc06155g  0.466
2020 Tendyck JC, Hepp A, Würthwein EU, Uhl W. New Reactivity Patterns in 3H-Phosphaallene Chemistry [Aryl-P=C=C(H)-tBu]: Hydroboration of the C=C Bond, Deprotonation and Trimerisation. Chemistry (Weinheim An Der Bergstrasse, Germany). 26: 15977-15988. PMID 32618025 DOI: 10.1002/chem.202002506  0.453
2020 Brand A, Hepp A, Würthwein EU, Uhl W. Tridentate Ligand with Three Carbanions as Donor Atoms: Formation of Dinuclear, Heptacyclic Complexes of Boron, Aluminum, or Gallium with B-C-B, Al-C-Al, or Ga-C-Ga Three-Center-Two-Electron Bonds. Inorganic Chemistry. 59: 5558-5563. PMID 32233410 DOI: 10.1021/acs.inorgchem.0c00254  0.552
2020 Tendyck JC, Klöcker H, Schürmann L, Würthwein EU, Hepp A, Layh M, Uhl W. Aspects of Phosphaallene Chemistry: Heat-Induced Formation of 1,2-Dihydrophosphetes by Intramolecular Nucleophilic Aromatic Substitution and Photochemical Generation of Tricyclic Phosphiranes. The Journal of Organic Chemistry. 85: 14315-14332. PMID 32022561 DOI: 10.1021/acs.joc.9b03056  0.468
2019 Pleschka D, Uebing M, Lange M, Hepp A, Wübker AL, Hansen MR, Würthwein EU, Uhl W. Al/P- and Ga/P-Based Frustrated Lewis Pairs and Electronically Unsaturated Substrates: Ring Cleavage and Ring Closure, C-C and C-N Bond Formation. Chemistry (Weinheim An Der Bergstrasse, Germany). 25: 9315-9325. PMID 31081975 DOI: 10.1002/chem.201901659  0.583
2019 Klöcker H, Tendyck JC, Keweloh L, Hepp A, Uhl W. 3H-Phosphaallenes Revisited: Facile Synthesis by Hydroalumination of Alkynylphosphines and β-Elimination, Stability and Trapping of Transient Species by Coordination to Transition Metal Atoms. Chemistry (Weinheim An Der Bergstrasse, Germany). 25: 4793-4807. PMID 30681211 DOI: 10.1002/chem.201806334  0.427
2019 Brand A, Uhl W. Sterically Constrained Bicyclic Phosphines: A Class of Fascinating Compounds Suitable for Application in Small Molecule Activation and Coordination Chemistry. Chemistry (Weinheim An Der Bergstrasse, Germany). 25: 1391-1404. PMID 30126018 DOI: 10.1002/chem.201803331  0.324
2018 Keweloh L, Aders N, Hepp A, Pleschka D, Würthwein EU, Uhl W. A P-H functionalized Al/P-based frustrated Lewis pair - hydrophosphination of nitriles, ring opening with cyclopropenones and evidence of P[double bond, length as m-dash]C double bond formation. Dalton Transactions (Cambridge, England : 2003). PMID 29893387 DOI: 10.1039/c8dt01836g  0.572
2018 Lange M, Tendyck JC, Wegener P, Hepp A, Würthwein EU, Uhl W. Reactions of an Aluminium/Phosphorus Frustrated Lewis Pair (FLP) with α,β-Unsaturated Carbonyl Compounds: FLPs as Efficient Two-Electron Reductants with the Formation of Enolates, a cis-Enediolate, and an Allene. Chemistry (Weinheim An Der Bergstrasse, Germany). 24: 12856-12868. PMID 29337388 DOI: 10.1002/chem.201706089  0.614
2017 Uhl W, Hentschel A, Brand A, Wegener P. A Sterically Constrained Tricyclic PC3 Phosphine - Coordination Behaviour and Insertion of Chalcogen Atoms into P-C Bonds. Angewandte Chemie (International Ed. in English). PMID 29171723 DOI: 10.1002/anie.201711373  0.441
2017 Pleschka D, Layh M, Rogel F, Uhl W. Structure and reactivity of an Al/P-based frustrated Lewis pair bearing relatively small substituents at aluminium. Philosophical Transactions. Series a, Mathematical, Physical, and Engineering Sciences. 375. PMID 28739968 DOI: 10.1098/rsta.2017.0011  0.542
2017 Backs J, Lange M, Possart J, Wollschläger A, Mück-Lichtenfeld C, Uhl W. Facile Modulation of FLP Properties: A Phosphinylvinyl Grignard Reagent and Ga/P- and In/P2 -Based Frustrated Lewis Pairs. Angewandte Chemie (International Ed. in English). PMID 28156031 DOI: 10.1002/anie.201612485  0.317
2017 Martinewski K, Holtrichter-Rößmann T, Rösener C, Hepp A, Würthwein EU, Uhl W. Cooperative Activation of Isocyanates by Al-N-Based Active Lewis Pairs and the Generation of a C Chain by Simultaneous Formation of Two C-C Bonds. Chemistry (Weinheim An Der Bergstrasse, Germany). 23: 6129-6141. PMID 28079943 DOI: 10.1002/chem.201604630  0.605
2016 Devillard M, Declercq R, Nicolas E, Ehlers AW, Backs J, Saffon-Merceron N, Bouhadir G, Slootweg JC, Uhl W, Bourissou D. A Significant but Constrained Geometry Pt→Al Interaction: Fixation of CO2 and CS2, Activation of H2 and PhCONH2. Journal of the American Chemical Society. PMID 26977772 DOI: 10.1021/Jacs.6B01320  0.358
2016 Klöcker H, Layh M, Hepp A, Uhl W. Hydroalumination of alkynyl-aminophosphines as a promising tool for the synthesis of unusual phosphines: P-N bond activation, a transient phosphaallene, a zwitterionic AlP2C2 heterocycle and a masked Al/P-based frustrated Lewis pair. Dalton Transactions (Cambridge, England : 2003). 45: 2031-43. PMID 26391528 DOI: 10.1039/c5dt02825f  0.552
2015 Honacker C, Qu ZW, Tannert J, Layh M, Hepp A, Grimme S, Uhl W. Functionalized alkynyl-chlorogermanes: hydrometallation, Ge-Cl bond activation, Ge-H bond formation and chlorine-tert-butyl exchange via a transient germyl cation. Dalton Transactions (Cambridge, England : 2003). PMID 26610394 DOI: 10.1039/C5Dt03918E  0.513
2015 Klöcker H, Roters S, Hepp A, Uhl W. Alkynyl functionalized Al/P-based frustrated Lewis pairs - aluminium alkynide elimination and evidence for the formation of 3H-phosphaallenes [R-P=C=C(H)-(t)Bu]. Dalton Transactions (Cambridge, England : 2003). 44: 12670-9. PMID 26084038 DOI: 10.1039/c5dt01607j  0.426
2015 Jin X, Willeke M, Lucchesi R, Daniliuc CG, Fröhlich R, Wibbeling B, Uhl W, Würthwein EU. Hydroalumination of Ketenimines and Subsequent Reactions with Heterocumulenes: Synthesis of Unsaturated Amide Derivatives and 1,3-Diimines. The Journal of Organic Chemistry. 80: 6062-75. PMID 26031425 DOI: 10.1021/acs.joc.5b00466  0.445
2015 Uhl W, Pelties S, Tannert J, Ravoo BJ, Würthwein EU. Germacyclobutenes: generation by 1,1-carbalumination or 1,1-carbagallation and their photophysical properties. Chemistry (Weinheim An Der Bergstrasse, Germany). 21: 2629-37. PMID 25522339 DOI: 10.1002/chem.201405739  0.557
2015 Uhl W, Tannert J, Honacker C, Layh M, Qu ZW, Risthaus T, Grimme S. Cooperative Ge-N Bond activation in aluminium-functionalised aminogermanes and spontaneous imine elimination via an intermediate germyl cation. Chemistry (Weinheim An Der Bergstrasse, Germany). 21: 2638-50. PMID 25521391 DOI: 10.1002/Chem.201405989  0.467
2014 Uhl W, Appelt C, Wollschläger A, Hepp A, Würthwein EU. An Al/P-based frustrated Lewis pair as an efficient ambiphilic ligand: coordination of boron trihalides, rearrangement, and formation of HBX₂ complexes (X = Br, I). Inorganic Chemistry. 53: 8991-9. PMID 25144381 DOI: 10.1021/ic5009126  0.394
2014 Uhl W, Bohnemann J, Kappelt B, Hepp A, Layh M. Hydrometallation of amino-trialkynylsilanes--intramolecular M-N interactions (M = Al, Ga) and potential activation of Si-N bonds. Dalton Transactions (Cambridge, England : 2003). 43: 14386-98. PMID 24968284 DOI: 10.1039/c4dt00922c  0.43
2013 Hengesbach F, Jin X, Hepp A, Wibbeling B, Würthwein EU, Uhl W. Activation of isocyanates and carbon dioxide by a monomeric aluminium hydrazide as an active Lewis pair. Chemistry (Weinheim An Der Bergstrasse, Germany). 19: 13901-9. PMID 24038438 DOI: 10.1002/chem.201302179  0.317
2013 Appelt C, Slootweg JC, Lammertsma K, Uhl W. Reaction of a P/Al-based frustrated Lewis pair with ammonia, borane, and amine-boranes: adduct formation and catalytic dehydrogenation. Angewandte Chemie (International Ed. in English). 52: 4256-9. PMID 23471587 DOI: 10.1002/Anie.201208746  0.326
2013 Uhl W, Würthwein EU. Novel Al-based FLP systems. Topics in Current Chemistry. 334: 101-19. PMID 23114496 DOI: 10.1007/128_2012_374  0.466
2013 Erdmann M, Rösener C, Holtrichter-Rößmann T, Daniliuc CG, Fröhlich R, Uhl W, Würthwein EU, Kehr G, Erker G. Functional group chemistry at intramolecular frustrated Lewis pairs: substituent exchange at the Lewis acid site with 9-BBN. Dalton Transactions (Cambridge, England : 2003). 42: 709-18. PMID 23014979 DOI: 10.1039/C2Dt31737K  0.361
2012 Roters S, Hepp A, Slootweg JC, Lammertsma K, Uhl W. Alkynide and acetonitrile activation by strained AlPC2 heterocycles. Chemical Communications (Cambridge, England). 48: 9616-8. PMID 22911118 DOI: 10.1039/C2Cc33300G  0.376
2012 Roters S, Appelt C, Westenberg H, Hepp A, Slootweg JC, Lammertsma K, Uhl W. Dimeric aluminum-phosphorus compounds as masked frustrated Lewis pairs for small molecule activation. Dalton Transactions (Cambridge, England : 2003). 41: 9033-45. PMID 22411491 DOI: 10.1039/C2Dt30080J  0.45
2012 Uhl W, Hepp A, Layh M, Rezaeirad B. The missing link in the coordination chemistry of hydrazines--a hydrazinetriide [N-N(Me)](3-) anion coordinated to five Al atoms. Chemical Communications (Cambridge, England). 48: 1799-801. PMID 22218427 DOI: 10.1039/c2cc16208c  0.344
2011 Uhl W, Kovert D, Layh M, Hepp A. Vinylgallium and alkyllithium compounds: transmetalation and generation of oligolithium cages. Chemistry (Weinheim An Der Bergstrasse, Germany). 17: 13553-61. PMID 22021130 DOI: 10.1002/chem.201102057  0.388
2011 Uhl W, Layh M, Rezaeirad B. Aluminum, gallium, and indium hydrazides and the generation of oligonuclear element-nitrogen cages: molecular intermediates on the way to element nitrides. Inorganic Chemistry. 50: 12275-83. PMID 21539316 DOI: 10.1021/ic200572q  0.302
2009 Uhl W, Claesener M, Hepp A, Jasper B, Vinogradov A, van Wüllen L, Köster TK. The influence of halogen substituents on the course of hydrogallation and hydroalumination reactions. Dalton Transactions (Cambridge, England : 2003). 10550-62. PMID 20023879 DOI: 10.1039/b913568e  0.481
2009 Uhl W, Reza Halvagar M, Claesener M. Reducing Ga-H and Ga-C bonds in close proximity to oxidizing peroxo groups: conflicting properties in single molecules. Chemistry (Weinheim An Der Bergstrasse, Germany). 15: 11298-306. PMID 19780106 DOI: 10.1002/chem.200900746  0.312
2009 Uhl W, Abel T, Hepp A, Nilges T, Rogel F, Würthwein EU, Ghavtadze N. The unique decomposition behavior of the dimeric dialkylaluminum hydrazide [(Me3C)2Al-N(H)-N(H)-Me]2-butane versus ammonia elimination. Inorganic Chemistry. 48: 752-9. PMID 19072532 DOI: 10.1021/ic8016134  0.348
2008 Uhl W, Bock HR, Claesener M, Layh M, Tiesmeyer I, Würthwein EU. cis/trans Isomerism of hydroalumination and hydrogallation products-reflections on stability and rearrangement mechanism. Chemistry (Weinheim An Der Bergstrasse, Germany). 14: 11557-64. PMID 19009572 DOI: 10.1002/chem.200801257  0.512
2008 Uhl W, Jana B. A persistent alkylaluminum peroxide: surprising stability of a molecule with strong reducing and oxidizing functions in close proximity. Chemistry (Weinheim An Der Bergstrasse, Germany). 14: 3067-71. PMID 18283706 DOI: 10.1002/chem.200701916  0.561
2008 Uhl W, Claesener M. Twofold hydrogallation of C triple bonds c triple bonds by H-GaCl(2)-synthesis of chelating Lewis acids and their application in adduct formation. Inorganic Chemistry. 47: 729-35. PMID 18081277 DOI: 10.1021/ic701928s  0.486
2008 Uhl W, Claesener M. Hydrogallation of alkynes with H-GaCl2: formation of organoelement dichlorogallium compounds potentially applicable as chelating Lewis acids. Inorganic Chemistry. 47: 4463-70. PMID 17665906 DOI: 10.1021/ic700767a  0.325
2007 Uhl W, Vinogradov A, Grimme S. C-H bond activation by hyperconjugation with Al-C bonds and by chelating coordination of the hydride ion. Journal of the American Chemical Society. 129: 11259-64. PMID 17705491 DOI: 10.1021/Ja073657U  0.592
2007 Uhl W, Claesener M, Haddadpour S, Jasper B, Hepp A. The reactions of dialkylgallium hydrides with tert-butylethynylbenzenes--a systematic investigation into the course of hydrogallation reactions. Dalton Transactions (Cambridge, England : 2003). 417-23. PMID 17213926 DOI: 10.1039/b614003c  0.425
1999 Uhl W, Breher F. Pentacarba-arachno-tridecaalane (AlMe) (CCH Ph) H with an Al C Skeleton-The First Polyhedral Carbaalane. Angewandte Chemie (International Ed. in English). 38: 1477-1479. PMID 29711579 DOI: 10.1002/(SICI)1521-3773(19990517)38:10<1477::AID-ANIE1477>3.0.CO;2-S  0.44
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